Off-campus University of Richmond users: To download campus access theses, please use the following link to log in to our proxy server with your university username and password.

Date of Award

2020

Document Type

Restricted Thesis: Campus only access

Degree Name

Bachelor of Science

Department

Chemistry

First Advisor

Dr. Wade Downey

Abstract

Ketones are easily converted to enol silanes in the presence of trimethylsilyl trifluoromethanesulfonate and an amine base, conditions that also result in the ionization of terminally silylated propargyl acetates. When these events occur in a single flask, the intermediates undergo an SN1 reaction to generate a B-propargyl ketone intermediate. Upon concentration in the presence of trace water, the intermediate cyclizes to provide 2- methylfurans in high yield. The use of various ketones and propargyl acetates allows for the synthesis of an extensive range of 2-methylfurans, which can be tested for biological activity.

Share

COinS